GEOC Programming: ACS Spring 2021 Meeting

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Macromolecular Chemistry: The Second Century

April 5-16 | Virtual

Time zone: Pacific Daylight Time (US and Canada)

Broadcast presentations through a virtual platform


Geochemistry Division Program

40 Years of High‐Resolution NMR Spectroscopy of Inorganic Solids

Oral Presentations: Monday (4/5) 9:00-3:35 pm PDT

Karl Mueller
Solids, surfaces, computers, and pencils: Targets and tools for solid‐state NMR

Mark E Smith
29Si and 27Al magic angle spinning NMR of oxynitride ceramics

Ian Farnan
High‐resolution nuclear magnetic resonance of highly radioactive solids: strategies and applications in radiation damage

Danielle Laurencin
Unraveling the structure and reactivity of interfacial oxygen sites thanks to oxygen‐17 mechanochemical labeling and high resolution NMR

Chia‐Hsin Chen
17O isotopic labeling of silica and titania using mechanochemistry: an investigation of enrichment mechanisms

Ieva Goldberga
Oxygen‐17 isotopic enrichment of calcium oxalate monohydrate phase

Eric Walter
In Situ Investigations of geochemical, extremophile and catalytic systems by high pressure: high temperature MAS‐NMR

Geoffrey Bowers
Linking NMR spectroscopy and computational molecular modeling to understand layer structure material

Sophia Hayes
29Si chemical shift tensors: From NMR experiments to computational prediction

Jorgen Skibsted
29Si and 27Al MAS NMR studies of Portland cements and zeolites

Mattias Eden
Solid state NMR and molecular dynamics simulation studies of phosphoserine‐doped calcium phosphate cements with bone‐adhesive properties

Christian Bonhomme
Hydroxyapatite revisited by DNP and spin diffusion: Natural abundance 43Ca DNP MAS and ultra high magnetic field (35T) 43Ca experiments, modeling and new mathematical treatment of dynamic nuclear polarization process

Oral Presentations: Tuesday (4/6) 9:00-11:50 am PDT

Pierre Florian
Getting the most information from the worst resolution: NMR of disordered solids

Cesar Leroy
In‐depth atomic‐scale structure and surface acidity description of aluminum oxide layers by ssNMR and DNP SENS spectroscopies

Randall Youngman
Enabling glass‐ceramic research with NMR

Hellmut Eckert
The glassy part of glass ceramics: Structural insights from solid state NMR

Brian Phillips
Insights from NMR spectroscopy on the diversity of boron defects in calcite

Yining Huang
High‐resolution SSNMR: Insights into the structure and chemistry of metal‐organic frameworks

Philip Grandinetti
Statistical earning of NMR tensors from 2D Si‐29 isotropic/anisotropic correlation nuclear magnetic resonance spectra of silicate glasses


Molecular Processes at Mineral‐Water Interfaces

Oral Presentations: Tuesday (4/6) 1:00-4:00 pm PDT

Marie Gaigeot
Silica‐water interfaces as a good platform/playfield for revealing hydrophilic to hydrophobic structural order of interfacial water

Jing Zhang
Multi‐technique approach on the adsorption of mono‐ and poly‐vanadate (V(V)O 3‐) onto hematite

Sang Soo Lee
Salinity dependent evolution of the electrical double layer at the muscovite (001) water interface Intermission

Ian Bourg
Dielectric spectra of water in charged clay interlayer nanopores

Somaiyeh Dadashi
Influence of the spatially heterogeneous charge distribution on A2l O3 (0001) on the interfacial organization of acetonitrile‐water mixtures

Bijoya Mandal
Probing the interfacial solvent environment by measuring the vibrational lifetime of SCN‐at the Al2O3 (0001)‐aqueous interface

Oral Presentations: Wednesday (4/7) 9:00-3:55 pm PDT

Susan Rempe
Differentiating aqueous halide ions, locally: F, Cl, Br, I

Jacquelyn Bracco
Cation sorption at the barite (001)‐ and (210)‐water interfaces

Inva Braha
Pb desorption at the barite (001)‐water interface

John Bargar
Importance of organic matter as a control over U(IV)‐ and Pb(II)‐surface interactions in natural sediments

Evert Elzinga
Trace metal sorption by green rust: Macroscopic and spectroscopic analyses

Elizabeth Tomaszewski
Organic matter adsorption and fractionation to ferrihydrite under different salinity conditions

Alon Rabinovich
Effect of phenolic organics on struvite precipitation from simulated dairy wastewater

Sebastien Kerisit
Molecular‐scale controls on heterogeneous nucleation and growth at mineral‐water interfaces

Peng Yang
Enhanced selenate uptake by lead co‐sorption at the barite (001)‐water interface

Ruiyu Wang
On the role of Alumina in the origin of life: Surface driven assembly of amino acids

Alicia Schuitemaker
Atomic structure and dynamics at the calcium carbonate (CaCO3) vaterite water interface

Anshuman Satpathy
U(VI) reduction by structural iron(II) present in montmorillonite

Logan Augustine
DFT + thermodynamics method to study inner‐sphere adsorption occurring at the mineral‐water interface

Poster Presentations: Wednesday (4/21) 9:00-10:00 am Pacific Time

Anand Kumar
Aqueous alteration of potassium‐rich feldspar and effects on its ice nucleation ability

Alicia Moya
Carbonate rocks reactivity across scales: elucidating the role of biominerals

Abhishek Soni
Heterogeneous ice nucleation on the muscovite mica surface

Anita Sanchez
Sorption of methylated arsenic onto mackinawite (FeS)

Ruiyu Wang
Water hydrophilic behavior at aqueous/alumina interfaces


Fundamental Reactions Driving Macroscopic Geochemical Processes

Oral Presentations: Thursday (4/8) 9:00-3:45pm PDT

Paul Fenter
Understanding extrinsic controls to mineral water interfacial reactivity

Alejandro Fernandez‐Martinez
Probing the structure and reactivity of iron and aluminum minerals towards rare earth elements in acid mine drainage

Eric Ferrage
Upscaling strategies for the analysis of water diffusion in clay porous media

David Cole
Nanopore confinement of C‐H‐O mixed‐volatile fluids relevant to subsurface energy systems

Alexis Navarre‐Sitchler
Connecting the dots between fluid transport, physical heterogeneity, and the lab‐field dissolution rate discrepancy

Anthony Ladd
Evolution of grain shapes by dissolution: Validation and upscaling of pore‐scale simulations

Hang Deng
Multi‐scale investigation of the dynamic evolution of mineral coating

Xin Gu
Investigating weathering in shale across scales by tracking pseudomorphic transformation of pyrite

James Kubicki
Density functional theory modeling of Ba2+ and SO 2‐ adsorption onto the quartz (101) surface

Lawrence Anovitz
Frustrated coulombic and cation size effects on boehmite aggregation: a tumbler small‐ and ultra‐small angle neutron scattering study

Li Li
From pores to watersheds: reactions at interfaces

Narasimhan Loganathan
Interaction of natural organic matter with smectite mineral surfaces: A combined experimental and simulation study

Emily Wei‐Hsin
Sun Molecular dynamics simulations of water thin films, contact angles, and capillary pressure in a quartz nanopore in the presence of CO2 and organic molecules

Juliane Weber
The influence of microstructure on mineral dissolution‐reprecipitation: The model systems of CaCO3‐CaMg(CO3)2 and CaCO3‐FeCO3

YoungJae Kim
Replacement of calcium carbonate polymorphs by cerussite

Poster Presentations: Wednesday (4/21) 9:00-10:00 am Pacific Time

Matthew Siebecker
Experimental redox kinetics of nanoparticulate manganese oxide (MnO2) and dissolved organic carbon: UV‐Vis study

Erin Berns
Proton: Binding model to simulate pH buffering in Arctic tundra soils


Biogeochemical Transformation in the Underground Environment – Natural Processes and Engineered Implementations for Contaminant Abatement

Oral Presentations: Friday (4/9) 9:00-4:00pm PDT

Matthew Ginder‐Vogel
Impact of dissolved organic matter on phenolic contaminant oxidation by manganese oxides

Matthew Berens
Assessment of 2,4‐Dinitroanisole transformation using compound specific isotope analysis after in situ chemical reduction of iron oxides

Kevin Hickey
Modeling the reduction of nitroaromatics and munition constituents by humic acid using quantum chemically computed reaction energies and quinone‐like functional groups

Arata Katayama
Alternate functionality of humin, a solid‐phase humic substance, as extracellular electron mediator in carbon dioxide‐reducing acetogenesis

Merritt Logan
Ultrahigh resolution mass spectrometry analysis of organic nitrogen released upon permafrost thaw

Holly Roth
Impact of beaver ponds on biogeochemical cycling of organic nitrogen within a fire‐impacted watershed

William Bahureksa
Wildfire severity impacts on chemical transformation of soil organic carbon and nitrogen

Samantha Fuchs
Geochemical and geomechanical alteration by acidic brine of artificially fractured sandstone under strain

Maedeh Soleimanifar
Utilization of cerium oxide and neodymium oxide nanoparticles by Methylobacterium extorquens (ATCCÂ 14718)

Poster Presentations: Wednesday (4/21) 9:00-10:00 am Pacific Time

Danhui Xin
Comparison of mediated electrochemical analysis and chemical redox titration for measuring the electron storage capacity of biochar


Reactive Transport Modeling: A Cutting‐Edge Tool for Investigating Coupled Processes

Oral Presentations: Friday (4/9) 1:00-4:00pm PDT

Young‐Shin Jun
Reactive transport modeling to decipher dissolution and nucleation at the interface of supercritical CO2‐brine‐cement

Sergi Molins
Expanding the role of pore‐scale reactive transport models to capture the multiscale evolution of fractured media

Qian Zhang
Investigation of reactive transport processes in a fractured dolostone via multi‐scale simulations

Lauren Beckingham
Improving understanding of mineral reaction rates and permeability evolution in porous media

Olubukola Ishola
Application of machine learning to predict hydraulic tortuosity of highly heterogeneous porous media

Vitalii Starchenko
Mineral precipitation in porous media: Quantification of X‐ray tomography data and pore‐scale reactive transport simulations

Adedapo Awolayo
Investigation of accessible reactive surface area for improved prediction of CO2 mineralization in basaltic aquifer rocks

Hang Wen
Climatic controls on organic carbon transformation and transport at the hillslope scale

Andrew Freiburger
A PHREEQC simulation of scaling during RO desalination

Mengnan Li
Higher‐order finite element multiphase reactive transport model for unstructured and fractured grids: benchmark studies, scaling analysis, and applications to CO2 sequestration

Poster Presentations: Wednesday (4/21) 9:00-10:00 am Pacific Time

Ecenur Bulur
Transport‐reaction modeling of particulate organic matter dynamics in riverbed sediments


Interfacial Reactions under Nano‐scale Confinement

Oral Presentations: Monday (4/12) 9:00-4:00pm PDT

Sophie Le Caer
Confined water in aluminosilicate nanotubes: Structure, dynamics and the importance of charge separation effects upon irradiation

Sylvie Roke
The interfacial structure of water under confinement

Ian Bourg
Coupled fluxes of water and ions (NaCl) during flow through silica nanopores

Yaguang Zhu
Solution pH in nanopores is controlled by ionic surface propensities

Ward Thompson
Dynamics and spectroscopy of liquids in nanoscale amorphous silica pores

Vicki Grassian
Interfacial reactions involving thin films of particles

Sebastien Kerisit
Diffusion controls on divalent metal silicate carbonation in confined water films

Ke Yuan
Understanding the nucleation and growth of barite by optical microscopy and X‐ray nanotomography

John Loring
Low temperature magnesite growth during forsterite carbonation in thin H2O films

David Cole
Probing the olivine‐water interface: Experimental and molecular simulation perspectives


Crystallization Pathways: New Perspectives on Nucleation, Growth & Dissolution of Natural & Synthetic Materials

Oral Presentations: Tuesday (4/13) 9:00-12:00pm PDT

Katherine Hull
Insights on shale iron leaching and secondary mineral crystallization through phase and morphology analysis

Maria Meza
Determination of solubility constants and thermodynamic variables for uranyl arsenate solids containing monovalent cations sodium (Na) and potassium (K)

Ian Bourg
Adsorption and aggregation of soil organic matter at the clay‐water interface

Bart Kahr
Helicoidal Growth and Charge Transport

Maria Sushko
Role of interfacial structure and dynamics in driving non‐classical crystallization

Tyler Schmidt
Metadynamics simulations of ion detachment from calcite (104)

Kristen Fichthorn
Kinetics of halide‐mediated Cu nanowire growth

Poster Presentations: Wednesday (4/21) 9:00-10:00 am Pacific Time

Connor Schmidt
Mesoscale structure of Ediacaran and synthetic dolomite spherulites

Yi Ren
Effects of pH on immersion freezing by kaolinite

Michela La Bella
Diffraction: tomography investigations on the hydration of gypsum plaster


Interfacial Reactions under Nano‐scale Confinement

Oral Presentations: Tuesday (4/13) 9:00-11:55am PDT

Laura Fumagalli
Direct measurement of the anomalously low dielectric constant of confined water

Derk Joester
Crystallization Kinetics of Amorphous Carbonates in Confinement

Young‐Shin Jun
Calcium phosphate’s nucleation kinetics and energy barrier in nanoscale confined organic spaces

Kevin Leung
Interplay of physically different properties leading to challenges in separating lanthanidecations ‐‐ an Ab Initio molecular dynamics and experimental study

Tina Nenoff
In situ PDF/DRIFTS Study of the role of water in Ag particle formation in zeolites

Anastasia Ilgen
Adsorption of lanthanides at nanoconfined silica and alumina‐water interfaces


Crystallization Pathways: New Perspectives on Nucleation, Growth & Dissolution of Natural & Synthetic Materials

Oral Presentations: Tuesday (4/13) 1:00-3:35pm PDT

R Lee Penn
Formation, growth, dissolution, and transformation of nanoparticles in reactive liquid media

Guomin Zhu
Self‐similar mesocrystals form via interface‐driven nucleation and assembly

Michel Sassi
Structure and composition of ferrihydrite nanoparticles from Ab Initio thermodynamics

Alireza Namayandeh
System chemistries control the formation and transformation kinetics of Fe13 like clusters

Si Chen
Observation and synthesis of exceptionally Fe‐deficient "hydrohematite" and "hydrogoethite"

Young‐Shin Jun
Nucleation kinetics and thermodynamics of iron(III) (hydr)oxide nanoparticles forming on quartz


Interfacial Reactions under Nano‐scale Confinement

Oral Presentations: Tuesday (4/13) 1:00-1:50pm PDT

Jeffery Greathouse
Synergistic effects of nanoconfinement and surface charge on iron adsorption on mesoporous silica

Michael Whittaker
Dynamic clay microstructures emerge via ion complexation waves at the mineral interface


Crystallization Pathways: New Perspectives on Nucleation, Growth & Dissolution of Natural & Synthetic Materials

Oral Presentations: Wednesday (4/14) 9:00-11:45am PDT

Xin Zhang
Unravel particle‐mediated crystallization pathways via using advanced transmission electron microscopy techniques

Qian Chen
In‐situ TEM based cinematography to elucidate crystallization pathways at the nanoscale

F. Marc Michel
Impacts of initial Ca/P on the formation and transformation of amorphous calcium phosphate

Rogier Besselink
High energy X‐ray Scattering revealing the short‐range order of a metastable proto‐CSH phase and its implications on cement nucleation

Yarong Qi
Role of organic foulants on the kinetics of silica scaling: Behavior and mechanisms

Andrew Lauer
Multi‐step nucleation in strontium sulfate: Reaction mechanisms and a hemihydrated precursor


General Geochemistry

Oral Presentations: Wednesday (4/14) 9:00-11:20am PDT

Qian Wang
Dynamic transformation of phosphorus and nitrogen during hydrothermal treatment (HT) of sewage sludge and resource recovery from HT process water

Chelsea Neil
Effects of water saturation on noble gas diffusion through zeolitic tuff

Hasini Senanayake
Simulations of the IR and raman spectra of water confined in amorphous silica slit pores

Hidemitsu Katsura
The variation of air radiation dose rates from December 2019 to March 2020 inside cabin flights between Tokyo and Singapore or Tokyo and Kuala Lumpur

Yunpo Li
Geochemical indicators in northeastern Pennsylvania groundwater are consistent with natural methane sources

Florence Ling
Modeling CaSiO3‐CO2 reactions and permeability evolution for sealing leakages from geologic carbon storage

Poster Presentations: Wednesday (4/21) 9:00-10:00 am Pacific Time

Samantha James
HF: Free extraction technique of particulate organic matter from sedimentary rocks

Boris Lau
Temperature effects on the interactions of soil organic matter with hematite and goethite: Perspectives on bulk and nano‐scale sorption

Amelia Bunnell
Sample preconcentration and matrix removal via SPE for the determination of dissolved hydrolyzable amino acids in estuarine samples via liquid chromatography tandem mass spectrometry

Reza Khalidy
Geochemical modeling applications and research hot spots ‐ a scientometric and critical review of 2019

Alejandro Briso
A simple geochemical approach to identify scenarios for managing drinking water treatment residuals (DWTRs)

Tiara Ogus
Phosphorus cycling and retention in agriculturally dominated stream ecosystems in semi‐arid Mediterranean climates


Crystallization Pathways: New Perspectives on Nucleation, Growth & Dissolution of Natural & Synthetic Materials

Oral Presentations: Wednesday (4/14) 1:00 - 3:15pm PDT

Yaguang Zhu
Roles of sulfate in the nucleation, growth, and Ostwald ripening of CaCO3 on quartz

Sebastian Mergelsberg
Nucleation of mixed‐cation amorphous carbonate precursors: Example of cadmium in ACC and vaterite

Christian Bonhomme
In situ description of biomineralization processes and pre‐crystalline phases studied by solid state NMR: The study case of hydrated calcium oxalates

Juan Diego Rodriguez‐Blanco
New insights into the mechanisms of bastnäsite formation


Reactivity & Transformation of Manganese Oxides in Natural and Engineering Systems

Oral Presentations: Thursday (4/15) 9:00-3:45pm PDT

Jeffrey Post
Raman spectroscopy identification and characterization of natural and synthetic manganese oxides

Zhenwei Gao
Photochemically‐induced co‐oxidation of Mn2+ and Co2+ and the formation of CoIII‐incorporated MnIV oxides

Young‐Shin Jun
Effects of reactive halogen species on the formation of photochemically‐induced abiotic MnIV oxides

Daniel Strongin
Redox chemistry and structural transformations relevant to birnessite as an electrocatalyst for water oxidation

James Kubicki
Macroscopic and molecular understanding of Np(V) sorption on the birnessite‐water interface

Martial Taillefert
Insights into the mechanism of reduction of manganese oxides by thiols and arsenite

Boyoung Song
Transmission electron microscopy (TEM) investigation of aggregate structures and their impacts on reactivity of manganese oxide mixtures

Matthew Fischel
Kinetics of arsenic oxidation by naturally formed manganese‐oxides

Yuanzhi Tang
Redox cycling driven transformation of layered manganese oxides to tunnel structures

Mengqiang Zhu
Mn(II)‐promoted phase transformation of manganese oxides

Peng Yang
Mn(II)‐driven redox transformation of layered Mn oxides in seawater

Seonyi Namgung
Adsorbed Mn(II) formed Mn oxide nano‐needles on the tip of goethite particles when exposed to oxygen

Jasquelin Pena
The fate of bioavailable carbon sources in presence of manganese oxides

Margaret Hinkle
Trace metal uptake by biogenic manganese oxides with structural variability: Connecting lessons from coal mine drainage remediation and the laboratory

Michael Zdilla
Experimental optimization of layered manganese oxide water‐oxidation catalysts by nano‐level organizational control guided by molecular dynamics and quantum calculation

Amritpal Singh Chaddha
Rock varnish: Potential future product

Poster Presentations: Wednesday (4/21) 9:00-10:00 am Pacific Time

Edwin Rivas Meraz
Remediation of mercury: Contaminated aquatic sediments with manganese(IV) oxide and activated carbon amendments


Engineered Nanomaterials and Synthetic Macromolecules in the Environment: Fate, Behavior, and Effects

Oral Presentations: Friday (4/16) 9:00-10:20am PDT

Eduardo Rodrigues
Uptake and accumulation of cerium oxide nanoparticles, as environmental contaminants, by soybean plants

Rafael Santos
Photodegradation of Quantum Dots: A New Kinetic Model and Significance of Structural Parameters

Pooya Paydary
Concluding Remarks


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